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The invention teaches a method for separating uranium and the transuranic actinides neptunium, plutonium, and americium from nitric acid solutions by co-crystallization upon lowering the temperature from 60 C to 20 C or lower.

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A novel strategy was developed to solve the limitations of the current sorbent systems in CO2 chemisorption in terms of energy consumption in CO2 release and improved CO2 uptake capacity.